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Lattice-driven chiral charge density wave state in 1T−TaS2

Manoj Singh1, Boning Yu1, James Huber1, Bishnu Sharma1, Ghilles Ainouche1, Ling Fu1, Jasper van Wezel2, and Michael C. Boyer1,*

  • 1Department of Physics, Clark University, Worcester, Massachusetts 01610, USA
  • 2Institute for Theoretical Physics Amsterdam, University of Amsterdam, Science Park 904,1098 XH Amsterdam, The Netherlands

  • *Author to whom correspondence should be addressed: mboyer@clarku.edu

Phys. Rev. B 106, L081407 – Published 19 August, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L081407

Abstract

We use scanning tunneling microscopy to study the domain structure of the nearly commensurate charge density wave (NC-CDW) state of 1T−TaS2. In our subangstrom characterization of the state, we find a continual evolution of the CDW lattice from domain wall to domain center, instead of a fixed CDW arrangement within a domain. Further, we uncover an intradomain chirality characterizing the NC-CDW state. Unlike the orbital-driven chirality previously observed in related transition-metal dichalcogenides, the chiral nature of the NC-CDW state in 1T−TaS2 appears driven by a strong coupling of the NC-CDW state to the lattice.

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