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  • Letter

Dirac nodal lines and nodal loops in the topological kagome superconductor CsV3Sb5

Zhanyang Hao1,2,*, Yongqing Cai1,2,*, Yixuan Liu1,2,*, Yuan Wang1,2,*, Xuelei Sui3, Xiao-Ming Ma1,2, Zecheng Shen1,2, Zhicheng Jiang4, Yichen Yang4 et al.

Wanling Liu4, Qi Jiang4, Zhengtai Liu4, Mao Ye4, Dawei Shen4, Yi Liu5, Shengtao Cui5, Jiabin Chen3, Le Wang1,2, Cai Liu1,2, Junhao Lin1, Jianfeng Wang6,3,†, Bing Huang3, Jia-Wei Mei1,2,7,†, and Chaoyu Chen1,2,†

  • 1Shenzhen Institute for Quantum Science and Engineering, and Department of Physics, Southern University of Science and Technology, Shenzhen 518055, China
  • 2International Quantum Academy, Shenzhen 518048, China
  • 3Beijing Computational Science Research Center, Beijing 100193, China
  • 4State Key Laboratory of Functional Materials for Informatics and Center for Excellence in Superconducting Electronics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, China
  • 5National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei 230029, China
  • 6School of Physics, Beihang University, Beijing 100191, China
  • 7Shenzhen Key Laboratory of Advanced Quantum Functional Materials and Devices, Southern University of Science and Technology, Shenzhen 518055, China

  • *These authors contributed equally to this work
  • †Corresponding authors: wangjf06@buaa.edu.cn, meijw@sustech.edu.cn, chency@sustech.edu.cn

Phys. Rev. B 106, L081101 – Published 2 August, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L081101

Abstract

The intertwining of charge order, superconductivity, and band topology has promoted the AV3Sb5 (A=K, Rb, Cs) family of materials to the center of attention in condensed matter physics. Underlying those mysterious macroscopic properties such as giant anomalous Hall conductivity (AHC) and chiral charge density wave is their nontrivial band topology. While there have been numerous experimental and theoretical works investigating the nontrivial band structure and especially the van Hove singularities, the exact topological phase of this family remains to be clarified. In this work, we identify CsV3Sb5 as a Dirac nodal line semimetal based on the observation of multiple Dirac nodal lines and loops close to the Fermi level. Combining photoemission spectroscopy and density functional theory, we identify two groups of Dirac nodal lines along the kz direction and one group of Dirac nodal loops in the A−H−L plane. These nodal loops are located at the Fermi level within the instrumental resolution limit. Importantly, our first-principles analyses indicate that these nodal loops may be a crucial source of the mysterious giant AHC observed. Our results not only provide a clear picture to categorize the band structure topology of this family of materials, but also suggest the dominant role of topological nodal loops in shaping their transport behavior.

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