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  • Letter

Noncollinear ferrimagnetism and anomalous Hall effects in Mn4N thin films

Yangkun He1,*, Simon Lenne1, Zsolt Gercsi1, Gwenael Atcheson1, Jack O'Brien1, Daniel Fruchart2, Karsten Rode1, and J. M. D. Coey1

  • 1School of Physics, CRANN, Trinity College, Dublin 2, Ireland
  • 2Department of QUEST, Institut Néel, CNRS and UGA, 38042, Grenoble Cedex 9, France

  • *heya@tcd.ie

Phys. Rev. B 106, L060409 – Published 24 August, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L060409

Abstract

Thin films of Mn4N and related ternary metallic perovskites with perpendicular anisotropy are interesting for spintronics, but their magnetic structures differ from the triangular ferrimagnetism of the bulk. A temperature-independent anomalous Hall conductivity of −90Ω–1cm–1 was found in Mn4N films, in addition to the normal temperature-dependent contribution. Based on known spin structures of bulk Mn3ZN compounds and the distance dependence of the Mn-Mn exchange for first- and second-neighbor Mn-Mn pairs, we propose a topological noncollinear spin structure for the Mn4N films with perpendicular anisotropy. The Letter shows how a small change in symmetry of the spin structure can influence the magnetotransport properties of frustrated ferrimagnetic films.

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