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Gaps in topological magnon spectra: Intrinsic versus extrinsic effects

Seung-Hwan Do1,*, Joseph A. M. Paddison1, Gabriele Sala2, Travis J. Williams3, Koji Kaneko4,5, Keitaro Kuwahara6, Andrew F. May1, Jiaqiang Yan1, Michael A. McGuire1 et al.

Matthew B. Stone3, Mark D. Lumsden3, and Andrew D. Christianson1,†

  • 1Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
  • 2Second Target Station, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
  • 3Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
  • 4Materials Sciences Research Center, Japan Atomic Energy Agency, Tokai, Ibaraki 319-1195, Japan
  • 5Advanced Science Research Center, Japan Atomic Energy Agency, Tokai, Ibaraki 319-1195, Japan
  • 6Institute of Quantum Beam Science, Ibaraki University, Mito, Ibaraki 310-8512, Japan

  • *seunghwando@gmail.com
  • †christiansad@ornl.gov

Phys. Rev. B 106, L060408 – Published 24 August, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L060408

Abstract

Determining and explaining the presence of a gap at a magnon crossing point is a critical step to characterize the topological properties of a material. An inelastic neutron scattering study of a single crystal is a powerful experimental technique to probe the magnetic excitation spectra of topological materials. Here, we show that when the scattering intensity rapidly disperses in the vicinity of a crossing point, such as a Dirac point, the apparent topological gap size is extremely sensitive to experimental conditions including sample mosaic, resolution, and momentum integration range. We demonstrate these effects using comprehensive neutron scattering measurements of CrCl3. Our measurements confirm the gapless nature of the Dirac magnon in CrCl3, but also reveal an artificial, i.e., extrinsic, magnon gap unless the momentum integration range is carefully controlled. Our study provides an explanation of the discrepancies between spectroscopic and first-principles estimates of Dirac magnon gap sizes and provides guidelines for accurate measurement of topological magnon gaps.

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