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Weak ferromagnetism in Tb(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 high-entropy oxide perovskite thin films

Alan Farhan1,*, Federico Stramaglia2, Maria Cocconcelli1,3, Nikolai Kuznetsov1, Lide Yao4, Armin Kleibert2, Cinthia Piamonteze2, and Sebastiaan van Dijken1

  • 1Department of Applied Physics, Aalto University School of Science, P.O. Box 15100, FI-00076 Aalto, Finland
  • 2Paul Scherrer Institute, Forschungsstrasse 111, 5232 Villigen PSI, Switzerland
  • 3Dipartimento di Fisica, Politecnico di Milano, 20133 Milano, Italy
  • 4Nanomicroscopy Center, Aalto University School of Science, P.O. Box 15100, FI-00076 Aalto, Finland

  • *alan.farhan@gmx.net

Phys. Rev. B 106, L060404 – Published 16 August, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L060404

Abstract

We have studied the structural and magnetic properties of Tb(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 (T5BO) high-entropy oxide perovskite (HEOP) thin films. Using synchrotron-based x-ray absorption spectroscopy, employing x-ray magnetic circular dichroism, we performed an element-sensitive study of epitaxial T5BO thin films. The measurements reveal a magnetic multiphase with variable ferromagnetic ordering of all transition metal elements, providing a promising route towards designer ferroic properties in Tb-based HEOP thin films.

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