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Electromagnetic origin of the microwave absorption response of Fe3O4 thin films

James Wampler1,*, Nelson Hua1, Roopali Kukreja1,2,3, Juan Gabriel Ramírez4, Ali C. Basaran1, Eric E. Fullerton2, Oleg Shpyrko1, and Ivan K. Schuller1

  • 1Department of Physics and Center for Advanced Nanoscience, University of California San Diego, La Jolla, California 92093, USA
  • 2Center for Memory and Recording Research, University of California San Diego, La Jolla, California 92093-0401, USA
  • 3Department of Materials Science Engineering, University of California Davis, Davis, California 95616, USA
  • 4Department of Physics, Universidad de los Andes, Bogotá 111711, Colombia

  • *Present address: National High Magnetic Field Laboratory, Los Alamos National Laboratory, Los Alamos, New Mexico 87544; corresponding author: jamespwampler@gmail.com

Phys. Rev. B 106, L060402 – Published 10 August, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L060402

Abstract

Low-field microwave absorption techniques are ultrasensitive, nondestructive methods for probing electric and magnetic properties of solids. Nonresonant low-field microwave absorption techniques such as magnetic field modulated microwave spectroscopy (MFMMS) can easily detect electromagnetic phase transitions in minute and inhomogeneous samples. While this technique can easily and almost selectively identify superconducting transitions, magnetic phase transitions produce more varied responses. Here, we present a technique to investigate the electric and magnetic properties of a sample with complex electromagnetic responses. This technique involves taking a series of magnetic hysteresis loops and magnetoresistance measurements. These can be compared to MFMMS data to identify features having electric or magnetic origin. This approach is applied to magnetite (Fe3O4), which possesses an electric, magnetic, and structural phase transition across its Verwey transition. By measuring high-quality Fe3O4 thin films in MFMMS and complementary techniques, the previously inscrutable MFMMS signal is analyzed. Furthermore, a model of the MFMMS signal can be calculated from the magnetic and electric data, which reproduces most of the features of the experimentally obtained MFMMS signal. This technique broadens the capabilities of MFMMS beyond the detection of superconductors.

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