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  • Letter

Signatures of electronic correlations and spin-susceptibility anisotropy in nuclear magnetic resonance

Stephen Carr1,2, Charles Snider1, D. E. Feldman1,2, Chandrasekhar Ramanathan3, J. B. Marston1,2, and V. F. Mitrović1

  • 1Department of Physics, Brown University, Providence, Rhode Island 02912-1843, USA
  • 2Brown Theoretical Physics Center, Brown University, Providence, Rhode Island 02912-1843, USA
  • 3Department of Physics and Astronomy, Dartmouth College, Hanover, New Hampshire 03755, USA

Phys. Rev. B 106, L041119 – Published 29 July, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L041119

Abstract

We present a methodology for probing the details of electronic susceptibility through minimally invasive nuclear magnetic resonance techniques. Specifically, we classify electron-mediated long-range interactions in an ensemble of nuclear spins by revealing their effect on simple spin echo experiments. We find that the pulse strength and applied field orientation dependence of these spin echo measurements resolves the spatial extent and anisotropy of electronic spin susceptibility. This Letter provides an alternate explanation to NMR results in superconducting and magnetically ordered systems. The methodology has direct applications for sensing and characterizing emergent electronic phases.

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