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Magnetic field induced Anderson localization in the orbital-selective antiferromagnet BaMn2Bi2

Takuma Ogasawara1, Kim-Khuong Huynh2,*, Stephane Yu Matsushita2, Motoi Kimata3, Time Tahara4, Takanori Kida4, Masayuki Hagiwara4, Denis Arčon5,6, and Katsumi Tanigaki2,7,†

  • 1Department of Physics, Graduate School of Science, Tohoku University, 6-3 Aoba, Aramaki, Aoba-ku, Sendai 980-8578, Miyagi, Japan
  • 2Advanced Institute for Materials Research (WPI-AIMR), Tohoku University, 1-1-2 Katahira, Aoba, Sendai, 980-8577 Miyagi, Japan
  • 3Institute for Materials Research, 1-1-2 Katahira, Aoba, Sendai, 980-8577 Miyagi, Japan
  • 4Center for Advanced High Magnetic Field Science, Graduate School Science, Osaka University, 11 Machikaneyama, Toyonaka, 560-0043 Osaka, Japan
  • 5Faculty of Mathematics and Physics, University of Ljubljana, Jadranska cesta 19, 1000 Ljubljana, Slovenia
  • 6Jozef Stefan Institute, Jamova cesta 39, 1000 Ljubljana, Slovenia
  • 7BAQIS, Building 3, No. 10 Xibeiwang East Road, Haidian District, Beijing 100193, China

  • *huynh.kim.khuong.b4@tohoku.ac.jp
  • †katsumi.tanigaki.c3@tohoku.ac.jp

Phys. Rev. B 106, L041114 – Published 25 July, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L041114

Abstract

We report a metal-insulator transition (MIT) in the half-filled multiorbital antiferromagnet (AFM) BaMn2Bi2 that is tunable by a magnetic field perpendicular to the AFM sublattices. Instead of an Anderson-Mott mechanism usually expected in strongly correlated systems, we find by scaling analyses that the MIT is driven by an Anderson localization. Electrical and thermoelectrical transport measurements in combination with electronic band calculations reveal a strong orbital-dependent correlation effect, where both weakly and strongly correlated 3d-derived bands coexist with decoupled charge excitations. Weakly correlated holelike carriers in the dxy-derived band dominate the transport properties and exhibit the Anderson localization, whereas other 3d bands show clear Mott-like behaviors with their spins ordered into AFM sublattices. The tuning role played by the perpendicular magnetic field supports a strong spin-spin coupling between itinerant holelike carriers and the AFM fluctuations, which is in sharp contrast to their weak charge coupling.

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