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Acoustic phonon dispersion of α−RuCl3

Blair W. Lebert1, Subin Kim1, Danil A. Prishchenko2, Alexander A. Tsirlin2,3, Ayman H. Said4, Ahmet Alatas4, and Young-June Kim1,*

  • 1Department of Physics, University of Toronto, Toronto, Ontario, Canada M5S 1A7
  • 2Department of Theoretical Physics and Applied Mathematics, Institute of Physics and Technology, Ural Federal University, Mira Str. 19, 620002 Ekaterinburg, Russia
  • 3Experimental Physics VI, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, 86135 Augsburg, Germany
  • 4Advanced Photon Source, Argonne National Laboratory, Lemont, Illinois 60439, USA

  • *youngjune.kim@utoronto.ca

Phys. Rev. B 106, L041102 – Published 5 July, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L041102

Abstract

Acoustic phonons have recently been posited as playing an integral role in explaining the half-quantized thermal Hall effect in α−RuCl3. Therefore, we present much needed inelastic x-ray scattering measurements of its acoustic phonon dispersion, along with calculations using the frozen-phonon method. We also discuss a temperature study which conclusively shows a first-order structural transition to a non-C2/m space group at low temperature. Together these results are an important backbone for future theoretical and experimental studies of α−RuCl3.

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