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Free energy of twisting spins in Mn3Sn

Xiaokang Li1,*, Shan Jiang1,2, Qingkai Meng1, Huakun Zuo1, Zengwei Zhu1,†, Leon Balents3,4, and Kamran Behnia2

  • 1Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China
  • 2Laboratoire de Physique et d'Étude des Matériaux (ESPCI - CNRS - Sorbonne Université), PSL Research University, 75005 Paris, France
  • 3Kavli Institute for Theoretical Physics, University of California, Santa Barbara, California 93106-4030, USA
  • 4Canadian Institute for Advanced Research, Toronto, Ontario, Canada

  • *lixiaokang@hust.edu.cn
  • †zengwei.zhu@hust.edu.cn

Phys. Rev. B 106, L020402 – Published 18 July, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L020402

Abstract

The magnetic free energy is usually quadratic in the magnetic field and depends on the mutual orientation of the magnetic field and the crystalline axes. Tiny in magnitude, this magnetocrystalline anisotropy energy (MAE) is nevertheless indispensable for the existence of permanent magnets. Here, we show that in Mn3Sn, a noncollinear antiferromagnet that has attracted much attention following the discovery of its large anomalous Hall effect, the free energy of the spins has superquadratic components, which drive the MAE. We experimentally demonstrate that the thermodynamic free energy includes terms odd in the magnetic field [F(H3)+F(H5)] and generating sixfold and 12-fold angular oscillations in the torque response. We show that they are quantitatively explained by theory, which can be used to quantify relevant energy scales (Heisenberg, Dzyaloshinskii-Moriya, Zeeman, and single-ion anisotropy) of the system. Based on the theory, we conclude that in contrast to common magnets, what drives the MAE in Mn3Sn is the field-induced deformation of the spin texture.

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