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  • Letter

Electronic states dressed by an out-of-plane supermodulation in the quasi-two-dimensional kagome superconductor CsV3Sb5

Yang Luo1,*, Shuting Peng1,*, Samuel M. L. Teicher2,*, Linwei Huai1,*, Yong Hu1,3, Yulei Han4,1, Brenden R. Ortiz2, Zuowei Liang1, Zhiyuan Wei1 et al.

Jianchang Shen1, Zhipeng Ou1, Bingqian Wang1, Yu Miao1, Mingyao Guo1, Makoto Hashimoto5, Donghui Lu5, Zhenhua Qiao1, Zhenyu Wang1,†, Stephen D. Wilson2,‡, Xianhui Chen1, and Junfeng He1,§

  • 1Department of Physics and CAS Key Laboratory of Strongly-coupled Quantum Matter Physics, University of Science and Technology of China, Hefei, Anhui 230026, China
  • 2Materials Department and California Nanosystems Institute, University of California Santa Barbara, Santa Barbara, California 93106, USA
  • 3Swiss Light Source, Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland
  • 4Department of Physics, Fuzhou University, Fuzhou, Fujian 350108, China
  • 5Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA

  • *These authors contributed equally to this work.
  • †zywang2@ustc.edu.cn
  • ‡stephendwilson@ucsb.edu
  • §jfhe@ustc.edu.cn

Phys. Rev. B 105, L241111 – Published 21 June, 2022

DOI: https://doi.org/10.1103/PhysRevB.105.L241111

Abstract

CsV3Sb5 has attracted much recent attention as the first quasi-two-dimensional (2D) kagome superconductor. While the kagome layers are 2D in nature, increasing evidence has pointed to the importance of out-of-plane correlation in this material. However, it remains unclear whether such correlation can change the fundamental electronic structure of the quasi-2D system. Here, we reveal this missing piece of information, using angle-resolved photoemission spectroscopy, complemented by scanning tunneling microscope measurements. The three-dimensional electronic structures in the high-temperature state are revealed, which agree well with density-functional theory calculations. Electron energy bands are observed in the low-temperature state that exhibit additional periodicities along the out-of-plane momentum. These results reveal a direct response to the out-of-plane electronic supermodulation in the single-particle spectral function of CsV3Sb5, thus establishing an electronic platform to examine emergent phenomena beyond 2D limit in kagome superconductors.

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