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X-ray diffraction study of phase transformation dynamics of Fe and Fe-Si alloys along the shock Hugoniot using an x-ray free electron laser

A. Krygier1,2,*, M. Harmand1, B. Albertazzi3, E. E. McBride4,5, K. Miyanishi6,7, D. Antonangeli1, Y. Inubushi7,8, R. Kodama6,9, M. Koenig3,9 et al.

T. Matsuoka10, G. Mogni1, F. Pietrucci1, A. M. Saitta1, T. Togashi7,8, Y. Umeda9,11, T. Vinci3, M. Yabashi7,8, T. Yabuuchi7,8, G. Fiquet1, and N. Ozaki6,9

  • 1Sorbonne Université, Muséum National d'Histoire Naturelle, UMR CNRS 7590, Institut de Minéralogie, de Physique des Matériaux, et de Cosmochimie (IMPMC), F-75005 Paris, France
  • 2Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550, USA
  • 3LULI, CNRS, CEA, Sorbonne Université, Ecole Polytechnique, Institut Polytechnique de Paris, F-91120 Palaiseau Cedex, France
  • 4European XFEL GmbH, Holzkoppel 4, D-22869 Schenefeld, Germany
  • 5SLAC National Accelerator Laboratory, 2575 Sand Hill Road, MS 19, Menlo Park, California 94025, USA
  • 6Institute for Laser Engineering, Osaka University, Suita, Osaka 565-0871, Japan
  • 7RIKEN Spring-8 Center, Sayo, Hyogo 679-5148, Japan
  • 8Japan Synchrotron Radiation Research Institute, Sayo, Hyogo 679-5198, Japan
  • 9Graduate School of Engineering, Osaka University, Suita, Osaka 565-0871, Japan
  • 10Open and Transdisciplinary Research Initiatives, Osaka University, Suita, Osaka 565-0871, Japan
  • 11Institute for Integrated Radiation and Nuclear Science, Kyoto University, Sennan, Osaka 590-0494, Japan

  • *krygier1@llnl.gov

Phys. Rev. B 105, L220102 – Published 7 June, 2022

DOI: https://doi.org/10.1103/PhysRevB.105.L220102

Abstract

The x-ray free electron laser (XFEL) enables probing a highly compressed material response at the subnanosecond timescale. We exploit the ultrafast XFEL pulse to combine reflection x-ray diffraction and laser-driven shock compression to perform a study of the phase transformation and stability in Fe and Fe-Si alloys. Our approach enables us to observe that solid-solid phase transformations occur in Fe and Fe-Si8.5wt% in ≤130 ps at ∼130 GPa; no transformation is observed in Fe-Si16wt% up to 110 GPa. Density functional theory calculations predict similar phase relations.

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