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Direct observation of moiré flat-band breakdown at the edge of magic-angle twisted bilayer graphene

Long-Jing Yin1,2,*, Ling-Hui Tong1,2, Yue-Ying Zhou1,2, Yang Zhang1,2, Yuan Tian1, Li Zhang1, Lijie Zhang1, and Zhihui Qin1,†

  • 1Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University, Changsha 410082, China
  • 2Research Institute of Hunan University in Chongqing, Chongqing 401120, China

  • *yinlj@hnu.edu.cn
  • †zhqin@hnu.edu.cn

Phys. Rev. B 105, L201405 – Published 19 May, 2022

DOI: https://doi.org/10.1103/PhysRevB.105.L201405

Abstract

Low-energy moiré flat bands in magic-angle twisted bilayer graphene (tBG) have demonstrated incredible potential to exhibit rich exotic quantum phenomena. Theoretically, the moiré flat bands of tBG are based on the extended structures, i.e., the moiré patterns with periodic boundary conditions. However, a fundamental question of whether the flat bands can exist in the graphene moiré patterns with a reduced structure symmetry, such as sample edges, remains unanswered. Here, via scanning tunneling microscopy and spectroscopy, we study the local electronic properties of magic-angle tBG near the sample terminated edge and report a direct observation of breakdown of the moiré flat bands. We show that the moiré electronic structures, including the low-energy flat bands, can sufficiently exist in a complete moiré spot, i.e., a moiré supercell, right at the edge even if the translational symmetry of the moiré patterns is broken in one direction. However, the flat-band characteristic is obviously absent in the incomplete moiré spots that are partly terminated by the edge. Our results indicate that a whole moiré spot is sufficient and indispensable for the generation of the effective moiré flat bands in tBG.

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