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Doping a moiré Mott insulator: A t−J model study of twisted cuprates

Xue-Yang Song, Ya-Hui Zhang, and Ashvin Vishwanath

  • Department of Physics, Harvard University, Cambridge, Massachusetts 02138, USA

Phys. Rev. B 105, L201102 – Published 4 May, 2022

DOI: https://doi.org/10.1103/PhysRevB.105.L201102

Abstract

We theoretically explore twisted cuprate multilayers, a moiré material family where the individual layers are themselves strongly correlated. We study the twisted t-J model, using a slave-boson mean field treatment that is compatible with Mott physics at small doping. Furthermore, we incorporate the interlayer tunneling form-factor dictated by the symmetry of the Cu dx2−y2 orbital. Including both these features leads to a phase diagram distinct from earlier weak-coupling treatments that predicted large gap spontaneous topological superconductors. Instead, we find that spontaneous time reversal (T) breaking occurs around twist angle of θ=45∘, but only in a narrow window. Moreover, a nearly gapless superconductor is obtained, whose spectroscopic features parallels that in monolayer cuprates, despite the broken time reversal and reflection symmetries. At smaller θ however, driving an interlayer current can lead to a gapped topological phase. The energy-phase relation of the interlayer Josephson junction displays notable double-Cooper-pair tunneling which dominates around 45∘. The θ dependence of the Josephson critical current and the Shapiro steps are consistent with recent experiments. Utilizing the moiré structure as a probe of correlation physics, e.g., the pair density wave state, is discussed.

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