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Quantum phase of the chromium spinel oxide HgCr2O4 in high magnetic fields

Shojiro Kimura1, Shusaku Imajo2, Masaki Gen2, Tsutomu Momoi3, Masayuki Hagiwara4, Hiroaki Ueda5, and Yoshimitsu Kohama2

  • 1Institute for Materials Research, Tohoku University, Katahira 2-1-1, Sendai 980-8577, Japan
  • 2Institute for Solid State Physics, University of Tokyo, Kashiwa 277-8531, Japan
  • 3Condensed Matter Theory Laboratory, RIKEN, Wako, Saitama 351-0198, Japan
  • 4Center for Advanced High Magnetic Field Science, Graduate School of Science, Osaka University, Toyonaka, Osaka 560-0043, Japan
  • 5Department of Chemistry, Graduate School of Science, Kyoto University, Kitashirakawa Oiwake-cho, Sakyo-ku, Kyoto 606-8502, Japan

Phys. Rev. B 105, L180405 – Published 9 May, 2022

DOI: https://doi.org/10.1103/PhysRevB.105.L180405

Abstract

In this study, we have performed the magnetocaloric effect and the specific heat measurements of chromium spinel oxide HgCr2O4, wherein the magnetic Cr3+ ions form a highly frustrated pyrochlore lattice with significant spin-lattice coupling. In addition to the known magnetic-field-induced phases, our thermodynamic measurements detect a quantum phase just before the saturation of the magnetization, which has not been expected from the classical theories of the pyrochlore lattice antiferromagnet with spin-lattice coupling. Based on recent theoretical model calculation, we discuss the possibility of a spin nematic state appearing for this quantum phase.

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