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  • Letter

Symmetry-allowed nonlinear orbital response across the topological phase transition in centrosymmetric materials

Margarita Davydova1,2, Maksym Serbyn2, and Hiroaki Ishizuka1,3

  • 1Department of Physics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, USA
  • 2IST Austria, Am Campus 1, 3400 Klosterneuburg, Austria
  • 3Department of Physics, Tokyo Institute of Technology, Meguro-ku, Tokyo 152-8551, Japan

Phys. Rev. B 105, L121407 – Published 17 March, 2022

DOI: https://doi.org/10.1103/PhysRevB.105.L121407

Abstract

Nonlinear optical responses are commonly used as a probe for studying the electronic properties of materials. For topological materials, studies thus far focused on photogalvanic electric currents, which are forbidden in centrosymmetric materials because they require broken inversion symmetry. In this Letter, we propose a class of symmetry-allowed responses for inversion-symmetric topological insulators with two doubly degenerate bands. We consider a specific example of such a response, the orbital current, and show that the sign of the response reflects the Z2 topological index, i.e., the orbital current changes sign at the transition between trivial and topological insulator phases. This is illustrated in two models of topological insulators: the Bernevig-Hughes-Zhang model and the 1T′ phase of transition metal dichalcogenides.

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