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Multiple strong topological gaps and hexagonal warping in Bi4Te3

Thais Chagas1, Omar A. Ashour2, Guilherme A. S. Ribeiro1, Wendell S. Silva3, Zhenglu Li2, Steven G. Louie2,*, Rogério Magalhães-Paniago1,†, and Yves Petroff3,‡

  • 1Department of Physics, Federal University of Minas Gerais, Avenida Presidente Antônio Carlos 6627, 31270-901, Belo Horizonte, Brazil
  • 2Department of Physics, University of California, Berkeley, California 94720, USA and Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 3Brazilian Synchrotron Light Laboratory, Center for Research in Energy and Materials, R. Giuseppe Máximo Scolfaro 10000, 13083-970, Campinas, Brazil

  • *sglouie@berkeley.edu
  • †rogerio.paniago0@gmail.com
  • ‡yves.petroff@gmail.com

Phys. Rev. B 105, L081409 – Published 17 February, 2022

DOI: https://doi.org/10.1103/PhysRevB.105.L081409

Abstract

The electronic topology of Bi4Te3, composed of alternating Bi2 and Bi2Te3 layers, is investigated by density functional theory and angle-resolved photoemission spectroscopy. We find, remarkably, that there are three adjacent strong topological gaps with associated protected surface states within a 2-eV range of the Fermi level. The existence of three consecutive Dirac cones in k space gives promise for alternative phenomena and applications, e.g., production of single photons with different energies (in the infrared and visible ranges) for multichannel transport of quantum information as well as multiple degrees of freedom in electron pumping for lasers. Additionally, a surface-state Fermi surface with strong hexagonal warping is observed.

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