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Quasiparticle coherence in the nematic state of FeSe

H. Pfau1,2,3,*, M. Yi4, M. Hashimoto5, T. Chen4, P.-C. Dai4, Z.-X. Shen1,6,7, S.-K. Mo2, and D. Lu5

  • 1Stanford Institute of Materials and Energy Science, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA
  • 2Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 3Department of Physics, The Pennsylvania State University, University Park, Pennsylvania 16802, USA
  • 4Department of Physics and Astronomy, Rice University, Houston, Texas 77005, USA
  • 5Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA
  • 6Department of Physics, Stanford University, Stanford, California 94305, USA
  • 7Geballe Laboratory for Advanced Materials, Department of Applied Physics, Stanford University, Stanford, California 94305, USA

  • *heike.pfau@psu.edu

Phys. Rev. B 104, L241101 – Published 2 December, 2021

DOI: https://doi.org/10.1103/PhysRevB.104.L241101

Abstract

Electronic nematicity is a ubiquitous phenomenon in iron-based superconductors but its origin is still debated. Most models consider either spin or orbital degrees of freedom as the driving force but typically do not take electronic correlations into account. However, mass enhancements, coherent-incoherent crossovers, and the strong orbital differentiation can only be understood using correlations in a Hund's metal framework. Here, we study the influence of nematicity on the quasiparticle coherence in detwinned FeSe using angle-resolved photoemission spectroscopy (ARPES). We compare photoemission spectral weight from dxz and dyz orbitals in the coherent quasiparticle peak and in the incoherent Hubbard band and find an anisotropy between the two orbitals. We interpret our observation in terms of a more coherent dxz orbital compared to the dyz orbital inside the nematic phase. This result is in contrast to earlier predictions of an incoherent dxz orbital and highlights the importance of electronic correlations in the description of nematicity.

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