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Superexchange dominates in magnetic topological insulators

Cezary Śliwa1,*, Carmine Autieri2,3, Jacek A. Majewski4, and Tomasz Dietl2,5,†

  • 1Institute of Physics, Polish Academy of Sciences, Aleja Lotnikow 32/46, PL-02668 Warsaw, Poland
  • 2International Research Centre MagTop, Institute of Physics, Polish Academy of Sciences, Aleja Lotnikow 32/46, PL-02668 Warsaw, Poland
  • 3Consiglio Nazionale delle Ricerche CNR-SPIN, UOS Salerno, I-84084 Fisciano (Salerno), Italy
  • 4Institute of Theoretical Physics, Faculty of Physics, University of Warsaw, ulica Pasteura 5, PL-02093 Warsaw, Poland
  • 5WPI-Advanced Institute for Materials Research, Tohoku University, Sendai 980-8577, Japan

  • *sliwa@ifpan.edu.pl
  • †dietl@MagTop.ifpan.edu.pl

Phys. Rev. B 104, L220404 – Published 6 December, 2021

DOI: https://doi.org/10.1103/PhysRevB.104.L220404

Abstract

It has been suggested that the enlarged spin susceptibility in topological insulators, described by interband Van Vleck's formalism, accounts for the ferromagnetism of bismuth-antimony topological chalcogenides doped with transition metal impurities. In contrast, earlier studies of HgTe and related topological systems pointed out that the interband analog of the Ruderman-Kittel-Kasuya-Yosida interaction (the Bloembergen-Rowland mechanism) leads to antiferromagnetic coupling between pairs of localized spins. Here, we critically revisit these two approaches, show their shortcomings, and elucidate why the magnitude of the interband contribution is small even in topological systems. From the proposed theoretical approach and our computational studies of magnetism in Mn-doped HgTe and CdTe, we conclude that in the absence of band carriers, the superexchange dominates and its sign depends on the coordination and charge state of magnetic impurities rather than on the topological class of the host material.

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