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  • Letter

Realization of quantum dipoles in triangular lattice crystal Ba3Yb(BO3)3

Rabindranath Bag1, Matthew Ennis1,*, Chunxiao Liu2,*, Sachith E. Dissanayake1, Zhenzhong Shi1, Jue Liu3, Leon Balents4, and Sara Haravifard1,5,†

  • 1Department of Physics, Duke University, Durham, North Carolina 27708, USA
  • 2Department of Physics, University of California, Santa Barbara, California 93106, USA
  • 3Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA
  • 4Kavli Institute for Theoretical Physics, University of California, Santa Barbara, California 93106, USA
  • 5Department of Mechanical Engineering and Materials Science, Duke University, Durham, North Carolina 27708, USA

  • *These authors contributed equally to this work.
  • †Email address: sara.haravifard@duke.edu

Phys. Rev. B 104, L220403 – Published 2 December, 2021

DOI: https://doi.org/10.1103/PhysRevB.104.L220403

Abstract

We investigate the thermodynamic properties of the ytterbium-based triangular lattice compound Ba3Yb(BO3)3. The results demonstrate the absence of any long-range ordering down to 56 mK. Analysis of the magnetization, susceptibility, and specific heat measurements suggests that Ba3Yb(BO3)3 may realize an S=12 quantum dipole lattice, in which the dominant interaction is the long-range dipole-dipole coupling on the geometrically frustrated triangular lattice, and exchange interactions are subdominant or negligible.

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