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  • Letter

Distorted 3Q state driven by topological-chiral magnetic interactions

Soumyajyoti Haldar1,*,†, Sebastian Meyer1,*,‡, André Kubetzka2, and Stefan Heinze1

  • 1Institute of Theoretical Physics and Astrophysics, University of Kiel, Leibnizstrasse 15, 24098 Kiel, Germany
  • 2Department of Physics, University of Hamburg, 20355 Hamburg, Germany

  • *These authors contributed equally to this work.
  • †haldar@physik.uni-kiel.de, haldar.physics@gmail.com
  • ‡Present address: Nanomat/Q-mat/CESAM, Université de Liège, B-4000 Sart Tilman, Belgium.

Phys. Rev. B 104, L180404 – Published 11 November, 2021

DOI: https://doi.org/10.1103/PhysRevB.104.L180404

Abstract

We predict the occurrence of unexpected magnetic ground states in ultrathin Mn films due to the frustration of higher-order interactions. Based on density functional theory we show that significant chiral-chiral interactions occur in hexagonal Mn monolayers due to large topological orbital moments which interact with the emergent magnetic field. Due to the competition with biquadratic and four-spin interactions superposition states of spin spirals such as the 2Q state or a distorted 3Q state arise. Simulations of spin-polarized scanning tunneling microscopy images suggest that the distorted 3Q state could be the magnetic ground state of a Mn monolayer on Re(0001).

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