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Nonlinear optical response of resonantly driven polaron-polaritons

Aleksi Julku1, Miguel. A. Bastarrachea-Magnani1,2, Arturo Camacho-Guardian3, and Georg M. Bruun1,4

  • 1Center for Complex Quantum Systems, Department of Physics and Astronomy, Aarhus University, Ny Munkegade, DK-8000 Aarhus C, Denmark
  • 2Departamento de Física, Universidad Autónoma Metropolitana-Iztapalapa, San Rafael Atlixco 186, C.P. 09340 CDMX, Mexico
  • 3T.C.M. Group, Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge CB3 0HE, United Kingdom
  • 4Shenzhen Institute for Quantum Science and Engineering and Department of Physics, Southern University of Science and Technology, Shenzhen 518055, China

Phys. Rev. B 104, L161301 – Published 11 October, 2021

DOI: https://doi.org/10.1103/PhysRevB.104.L161301

Abstract

Exciton polaritons in two-dimensional semiconductors inside microcavities are powerful platforms to explore hybrid light-matter quantum systems. Here, we study a macroscopic coherent population of the lowest energy state of polaron-polaritons, which are quasiparticles formed by the dressing of exciton polaritons by particle-hole excitations in a surrounding electron gas. Using a nonperturbative many-body theory to describe exciton-electron correlations combined with a nonequilibrium theory for the macroscopically populated state, we show that the electrons strongly affect the collective properties of the polaron-polaritons. This stems from the dependence of the polaron-polariton energy and the interaction between them on the electron density, which leads to strong nonlinearities. We identify stable and unstable regimes of the polaron-polaritons by calculating its excitation spectrum, and show that they result in prominent hysteresis effects when the electron density is varied. Our results should be readily observable using present experimental technology.

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