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Multiple energy scales and anisotropic energy gap in the charge-density-wave phase of the kagome superconductor CsV3Sb5

Kosuke Nakayama1,2,*,†, Yongkai Li3,4,*, Takemi Kato1, Min Liu3,4, Zhiwei Wang3,4,†, Takashi Takahashi1,5,6, Yugui Yao3,4, and Takafumi Sato1,5,6,7,†

  • 1Department of Physics, Faculty of Science, Tohoku University, Sendai 980-8578, Japan
  • 2Precursory Research for Embryonic Science and Technology (PRESTO), Japan Science and Technology Agency (JST), Tokyo 102-0076, Japan
  • 3Centre for Quantum Physics, Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement (MOE), School of Physics, Beijing Institute of Technology, Beijing 100081, China
  • 4Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic Systems, Beijing Institute of Technology, Beijing 100081, China
  • 5Center for Spintronics Research Network, Tohoku University, Sendai 980-8577, Japan
  • 6WPI Research Center, Advanced Institute for Materials Research, Tohoku University, Sendai 980-8577, Japan
  • 7International Center for Synchrotron Radiation Innovation Smart (SRIS), Tohoku University, Sendai 980-8577, Japan

  • *These authors contributed equally to this work.
  • †Corresponding authors: k.nakayama@arpes.phys.tohoku.ac.jp; zhiweiwang@bit.edu.cn; t-sato@arpes.phys.tohoku.ac.jp

Phys. Rev. B 104, L161112 – Published 21 October, 2021

DOI: https://doi.org/10.1103/PhysRevB.104.L161112

Abstract

Kagome metals AV3Sb5 (A=K, Rb, and Cs) exhibit superconductivity at 0.9–2.5 K and charge-density wave (CDW) at 78–103 K. Key electronic states associated with the CDW and superconductivity remain elusive. Here, we investigate low-energy excitations of CsV3Sb5 by angle-resolved photoemission spectroscopy. We found an energy gap of 50–70 meV at the Dirac-crossing points of linearly dispersive bands, pointing to an importance of spin-orbit coupling. We also found a signature of strongly Fermi-surface and momentum-dependent CDW gap characterized by the larger energy gap of maximally 70 meV for a band forming a saddle point around the M point, the smaller (0–18 meV) gap for a band forming massive Dirac cones and a zero gap at the Γ/A-centered electron pocket. The observed highly anisotropic CDW gap which is enhanced around the M point signifies an importance of scattering channel connecting the saddle points, laying foundation for understanding the nature of CDW and superconductivity in AV3Sb5.

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