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Spin-scattering asymmetry at half-metallic-ferromagnet|ferromagnet interface

Y. Fujita1,*, Y. Miura2, T. Sasaki2, T. Nakatani2, K. Hono2, and Y. Sakuraba2,†

  • 1International Center for Young Scientists, National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan
  • 2Research Center for Magnetic and Spintronic Materials, National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan

  • *FUJITA.Yuichi@nims.go.jp
  • †SAKURABA.Yuya@nims.go.jp

Phys. Rev. B 104, L140403 – Published 8 October, 2021

DOI: https://doi.org/10.1103/PhysRevB.104.L140403

Abstract

We study spin-scattering asymmetry at the interface of two ferromagnets (FMs) based on a half-metallic Co2Fe0.4Mn0.6Si (CFMS)/CoFe interface. First-principles ballistic transport calculations based on Landauer formula for (001)-CoFe/CFMS/CoFe indicate strong spin-dependent conductance at the CFMS/CoFe interface, suggesting a large interface spin-scattering asymmetry coefficient (γ). Fully epitaxial current-perpendicular-to-plane giant magnetoresistance (CPP-GMR) pseudo-spin-valve (PSV) devices involving CoFe/CFMS/Ag/CFMS/CoFe structures exhibit an enhancement in MR output owing to the formation of the CFMS/CoFe interface at room temperature (RT). This is well reproduced qualitatively by a simulation based on a generalized two-current series-resistor model with considering the presence of γ at the CFMS/CoFe interface, half-metallicity of CFMS, and combinations of terminated atoms at the interfaces in the CPP-GMR PSV structure. We show direct evidence for a large γ at a half-metallic FM/FM interface and its impact on the CPP-GMR effect even at RT.

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