- Letter
- Open Access
Symmetry-controlled singlet-triplet transition in a double-barrier quantum ring
Phys. Rev. B 104, L081409 – Published 25 August, 2021
DOI: https://doi.org/10.1103/PhysRevB.104.L081409
Abstract
We engineer a system of two strongly confined quantum dots to gain reproducible electrostatic control of the even-electron spin at zero magnetic field. Coupling the dots in a tight ring-shaped potential with two tunnel barriers, we demonstrate that an electric field can switch the electron ground state between a singlet and a triplet configuration. Comparing our experimental cotunneling spectroscopy data to a full many-body treatment of interacting electrons in a double-barrier quantum ring, we find excellent agreement in the evolution of many-body states with electric and magnetic fields. The calculations show that the singlet-triplet energy crossover, not found in conventionally coupled quantum dots, is made possible by the ring-shaped geometry of the confining potential.
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References (34)
- D. Loss and D. P. DiVincenzo, Phys. Rev. A 57, 120 (1998).
- D. D. Awschalom, L. C. Bassett, A. S. Dzurak, E. L. Hu, and J. R. Petta, Science 339, 1174 (2013).
- C. Kloeffel and D. Loss, Annu. Rev. Condens. Matter Phys. 4, 51 (2013).
- R. Bulla, T. A. Costi, and T. Pruschke, Rev. Mod. Phys. 80, 395 (2008).
- J. R. Petta, A. C. Johnson, J. M. Taylor, E. A. Laird, A. Yacoby, M. D. Lukin, C. M. Marcus, M. P. Hanson, and A. C. Gossard, Science 309, 2180 (2005).
- B. M. Maune, M. G. Borselli, B. Huang, T. D. Ladd, P. W. Deelman, K. S. Holabird, A. A. Kiselev, I. Alvarado-Rodriguez, R. S. Ross, A. E. Schmitz, M. Sokolich, C. A. Watson, M. F. Gyure, and A. T. Hunter, Nature (London) 481, 344 (2012).
- M. D. Reed, B. M. Maune, R. W. Andrews, M. G. Borselli, K. Eng, M. P. Jura, A. A. Kiselev, T. D. Ladd, S. T. Merkel, I. Milosavljevic, E. J. Pritchett, M. T. Rakher, R. S. Ross, A. E. Schmitz, A. Smith, J. A. Wright, M. F. Gyure, and A. T. Hunter, Phys. Rev. Lett. 116, 110402 (2016).
- N. Roch, S. Florens, V. Bouchiat, W. Wernsdorfer, and F. Balestro, Nature (London) 453, 633 (2008).
- J. C. Estrada Saldaña, A. Vekris, G. Steffensen, R. Žitko, P. Krogstrup, J. Paaske, K. Grove-Rasmussen, and J. Nygård, Phys. Rev. Lett. 121, 257701 (2018).
- D. Bouman, R. J. J. van Gulik, G. Steffensen, D. Pataki, P. Boross, P. Krogstrup, J. Nygård, J. Paaske, A. Pályi, and A. Geresdi, Phys. Rev. B 102, 220505(R) (2020).
- S. M. Reimann and M. Manninen, Rev. Mod. Phys. 74, 1283 (2002).
- R. Hanson, L. P. Kouwenhoven, J. R. Petta, S. Tarucha, and L. M. K. Vandersypen, Rev. Mod. Phys. 79, 1217 (2007).
- S. Tarucha, D. G. Austing, T. Honda, R. J. van der Hage, and L. P. Kouwenhoven, Phys. Rev. Lett. 77, 3613 (1996).
- J. Schmid, J. Weis, K. Eberl, and K. v. Klitzing, Phys. Rev. Lett. 84, 5824 (2000).
- A. Kogan, G. Granger, M. A. Kastner, D. Goldhaber-Gordon, and H. Shtrikman, Phys. Rev. B 67, 113309 (2003).
- F. Martins, F. K. Malinowski, P. D. Nissen, S. Fallahi, G. C. Gardner, M. J. Manfra, C. M. Marcus, and F. Kuemmeth, Phys. Rev. Lett. 119, 227701 (2017).
- F. K. Malinowski, F. Martins, T. B. Smith, S. D. Bartlett, A. C. Doherty, P. D. Nissen, S. Fallahi, G. C. Gardner, M. J. Manfra, C. M. Marcus, and F. Kuemmeth, Phys. Rev. X 8, 011045 (2018).
- W. Liang, M. Bockrath, and H. Park, Phys. Rev. Lett. 88, 126801 (2002).
- C. H. L. Quay, J. Cumings, S. J. Gamble, R. dePicciotto, H. Kataura, and D. Goldhaber-Gordon, Phys. Rev. B 76, 245311 (2007).
- R. J. Warburton, C. Schaeflein, D. Haft, F. Bickel, A. Lorke, K. Karrai, J. M. Garcia, W. Schoenfeld, and P. M. Petroff, Nature (London) 405, 926 (2000).
- A. Fuhrer, T. Ihn, K. Ensslin, W. Wegscheider, and M. Bichler, Phys. Rev. Lett. 91, 206802 (2003).
- J. Kyriakidis, M. Pioro-Ladriere, M. Ciorga, A. S. Sachrajda, and P. Hawrylak, Phys. Rev. B 66, 035320 (2002).
- T. Hatano, S. Amaha, T. Kubo, Y. Tokura, Y. Nishi, Y. Hirayama, and S. Tarucha, Phys. Rev. B 77, 241301(R) (2008).
- M. Nilsson, F. V. Boström, S. Lehmann, K. A. Dick, M. Leijnse, and C. Thelander, Phys. Rev. Lett. 121, 156802 (2018).
- G. Burkard, D. Loss, and D. P. DiVincenzo, Phys. Rev. B 59, 2070 (1999).
- J. Planelles, F. Rajadell, and J. I. Climente, Nanotechnology 18, 375402 (2007).
- M. Nilsson, I.-J. Chen, S. Lehmann, V. Maulerova, K. A. Dick, and C. Thelander, Nano Lett. 17, 7847 (2017).
- C. Thelander, M. Nilsson, F. Viñas Boström, A. Burke, S. Lehmann, K. A. Dick, and M. Leijnse, Phys. Rev. B 98, 245305 (2018).
- H. Potts, M. Leijnse, A. Burke, M. Nilsson, S. Lehmann, K. A. Dick, and C. Thelander, Phys. Rev. B 101, 115429 (2020).
- W. G. van der Wiel, S. De Franceschi, J. M. Elzerman, T. Fujisawa, S. Tarucha, and L. P. Kouwenhoven, Rev. Mod. Phys. 75, 1 (2002).
- H. Potts, I.-J. Chen, A. Tsintzis, N. Malin, S. Lehmann, K. A. Dick, M. Leijnse, and C. Thelander, Nat. Commun. 10, 5740 (2019).
- T. Jespersen, K. Grove-Rasmussen, J. Paaske, K. Muraki, J. Nygard, and K. Flensberg, Nat. Phys. 7, 348 (2011).
- See Supplemental Material at http://link.aps.org/supplemental/10.1103/PhysRevB.104.L081409 for additional experimental results and details on the modelling, which includes Ref. [34].
- C. D. Boor, A Practical Guide to Splines (Springer, Berlin, 1978), Vol. 27.