- Letter
Two-dimensional ferromagnetic spin-orbital excitations in honeycomb
Phys. Rev. B 104, L020411 – Published 20 July, 2021
DOI: https://doi.org/10.1103/PhysRevB.104.L020411
Abstract
is a ferromagnet with planar honeycomb sheets of bonded ions held together by van der Waals forces. We apply neutron spectroscopy to measure the two-dimensional () magnetic excitations in the ferromagnetic phase, finding two energetically gapped () and dispersive excitations. We apply a multilevel spin-wave formalism to describe the spectra in terms of two coexisting domains hosting differing orbital ground states built from contrasting distorted octahedral environments. This analysis fits a common nearest-neighbor in-plane exchange coupling () between sites. The distorted local crystalline electric field combined with spin-orbit coupling provides the needed magnetic anisotropy for spatially long-ranged two-dimensional ferromagnetism in .