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Quantum critical phenomena in a spin-12 frustrated square lattice with spatial anisotropy

H. Yamaguchi1, Y. Iwasaki2, Y. Kono3, T. Okubo4, S. Miyamoto1, Y. Hosokoshi1, A. Matsuo5, T. Sakakibara5, T. Kida6 et al.

M. Hagiwara6

  • 1Department of Physical Science, Osaka Prefecture University, Osaka 599-8531, Japan
  • 2Center for Advanced High Magnetic Field Science (AHMF), Graduate School of Science, Osaka University, Osaka 560-0043, Japan
  • 3Department of Physics, Chuo University, Tokyo 112-8551, Japan
  • 4Department of Physics, the University of Tokyo, Tokyo 113-0033, Japan
  • 5Institute for Solid State Physics, the University of Tokyo, Chiba 277-8581, Japan
  • 6Center for Advanced High Magnetic Field Science (AHMF), Graduate School of Science, Osaka University, Osaka 560-0043, Japan

Phys. Rev. B 103, L220407 – Published 15 June, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L220407

Abstract

We present a model compound with a spin-12 spatially anisotropic frustrated square lattice, in which three antiferromagnetic interactions and one ferromagnetic interaction are competing. We observe an unconventional gradual increase in the low-temperature magnetization curve reminiscent of the quantum critical behavior between gapped and gapless phases. In addition, the specific heat and electron spin resonance signals indicate one-dimensional characteristics. These results demonstrate quantum critical behavior associated with one dimensionalization caused by frustrated interactions in the spin-12 spatially anisotropic square lattice.

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