Export citation

Export citation

Choose format for download:

Download Citation
  • Letter

Condensation of collective polar vortex modes

Tiannan Yang1,*, Cheng Dai1, Qian Li2, Haidan Wen3, and Long-Qing Chen1,†

  • 1Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, USA
  • 2State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China
  • 3Advanced Photon Source, Argonne National Laboratory, Lemont, Illinois 60439, USA

  • *tuy123@psu.edu
  • †lqc3@psu.edu

Phys. Rev. B 103, L220303 – Published 15 June, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L220303

Abstract

The dynamics of extended objects such as domain walls, domain bubbles, vortex structures, etc., can be described by their equations of motion associated with their effective mass and spring constant. Here we analytically derive the equations of motion for the polarization dynamics and elastodynamics for the structural responses of ferroelectric polar vortices, and theoretically extract their effective mass, spring constant, and mode frequencies. We demonstrate two subterahertz phonon modes and predicted their frequencies, both consistent with our recent experimental measurements and phase-field simulations. We show that elastic modulation of the energy function and spring constants leads to a condensation of a collective mode upon a second-order structural transition from symmetric to asymmetric vortices at a critical strain, analogous to the ferroelectric soft phonon mode at a ferroelectric transition. The present work offers a theoretical framework for predicting and manipulating the ultrafast collective dynamics of polar nanostructures.

Physics Subject Headings (PhySH)

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation