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Quantum transport of topological spin solitons in a one-dimensional organic ferroelectric

S. Imajo1,*, A. Miyake1, R. Kurihara1, M. Tokunaga1, K. Kindo1, S. Horiuchi2, and F. Kagawa3,4

  • 1Institute for Solid State Physics, University of Tokyo, Kashiwa, Chiba 277-8581, Japan
  • 2Research Institute of Advanced Electronics and Photonics (RIAEP), National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba 305-8565, Japan
  • 3RIKEN Center for Emergent Matter Science (CEMS), Wako 351-0198, Japan
  • 4Department of Applied Physics, University of Tokyo, Tokyo 113-8656, Japan

  • *imajo@issp.u-tokyo.ac.jp

Phys. Rev. B 103, L201117 – Published 21 May, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L201117

Abstract

We report the dielectric, magnetic, and ultrasonic properties of a one-dimensional organic salt TTF−QBr3I. These indicate that TTF−QBr3I shows a ferroelectric spin-Peierls (FSP) state in a quantum critical regime. In the FSP state, coupling of charge, spin, and lattice leads to emergent excitation of spin solitons as topological defects. Amazingly, the solitons are highly mobile even at low temperatures, although they are normally stationary because of pinning. Our results suggest that strong quantum fluctuations enhanced near a quantum critical point enable soliton motion governed by athermal relaxation. This indicates the realization of quantum topological transport at ambient pressure.

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