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  • Letter

Pseudogap metal induced by long-range Coulomb interactions

K. Driscoll, A. Ralko, and S. Fratini*

  • Institut Néel, Centre National de la Recherche Scientifique and Université Grenoble Alpes, 38042 Grenoble, France

  • *simone.fratini@neel.cnrs.fr

Phys. Rev. B 103, L201106 – Published 7 May, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L201106

Abstract

In correlated electron systems the metallic character of a material can be strongly suppressed near an integer concentration of conduction electrons as Coulomb interactions forbid the double occupancy of local atomic orbitals. While the Mott-Hubbard physics arising from such on-site interactions has been largely studied, several unexplained phenomena observed in correlated materials challenge this description and call for the development of new ideas. Here we explore a general route for obtaining correlated behavior that is decidedly different from the spin-related Mott-Hubbard mechanism and instead relies on the presence of unscreened, long-range Coulomb interactions. We find a pseudogap metal phase characterized by a divergent quasiparticle mass and the opening of a Coulomb pseudogap in the electronic spectrum. The destruction of the Fermi-liquid state occurs because the electrons move in a nearly frozen, disordered charge background, as collective charge rearrangements are drastically slowed down by the frustrating nature of long-range potentials on discrete lattices. The present pseudogap metal realizes an early conjecture by Efros, that a soft Coulomb gap should appear for quantum lattice electrons with strong unscreened interactions due to self-generated randomness.

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