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  • Letter

Magnetic correlations in the semimetallic hyperkagome iridate Na3Ir3O8

G. Simutis1,*, T. Takayama2,3, Q. Barthélemy1, F. Bert1, H. Takagi2,3, and P. Mendels1

  • 1Laboratoire de Physique des Solides, Paris-Saclay University and CNRS, France
  • 2Institute for Functional Matter and Quantum Technologies, University of Stuttgart, Germany
  • 3Max Planck Institute for Solid State Research, Stuttgart, Germany

  • *gediminas.simutis@universite-paris-saclay.fr

Phys. Rev. B 103, L100404 – Published 8 March, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L100404

Abstract

We present a microscopic study of a doped quantum spin liquid candidate, the hyperkagome Na3Ir3O8 compound, by using Na23 NMR. We determine the intrinsic behavior of the uniform q = 0 susceptibility via shift measurements and the dynamical response by probing the spin-lattice relaxation rate. Throughout the studied temperature range, the susceptibility is consistent with a semimetal behavior, though with electronic bands substantially modified by correlations. Remarkably, the antiferromagnetic fluctuations present in the insulating parent compound Na4Ir3O8 survive in the studied compound. The spin dynamics are consistent with 120∘ excitation modes displaying short-range correlations.

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