- Letter
Magnetic correlations in the semimetallic hyperkagome iridate
Phys. Rev. B 103, L100404 – Published 8 March, 2021
DOI: https://doi.org/10.1103/PhysRevB.103.L100404
Abstract
We present a microscopic study of a doped quantum spin liquid candidate, the hyperkagome compound, by using NMR. We determine the intrinsic behavior of the uniform q = 0 susceptibility via shift measurements and the dynamical response by probing the spin-lattice relaxation rate. Throughout the studied temperature range, the susceptibility is consistent with a semimetal behavior, though with electronic bands substantially modified by correlations. Remarkably, the antiferromagnetic fluctuations present in the insulating parent compound survive in the studied compound. The spin dynamics are consistent with excitation modes displaying short-range correlations.