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Magnetic excitations in long-range stripe-ordered Pr2NiO4+δ

Avishek Maity1,*, Rajesh Dutta2,3,†, Anna Marsicano4, Andrea Piovano5, J. Ross Stewart6, and Werner Paulus4,‡

  • 1Heinz Maier-Leibnitz Zentrum (MLZ), Technische Universität München, 85747 Garching, Germany
  • 2Institut für Kristallographie, RWTH Aachen Universität, 52066 Aachen, Germany
  • 3Jülich Centre for Neutron Science (JCNS) at Heinz Maier-Leibnitz Zentrum (MLZ), 85747 Garching, Germany
  • 4Institut Charles Gerhardt Montpellier, Université de Montpellier, CNRS-ENSCM, 34095 Montpellier, France
  • 5Institut Laue-Langevin, 71 Avenue des Martyrs, 38000 Grenoble, France
  • 6ISIS Neutron and Muon Source, Rutherford Appleton Laboratory, Didcot OX11 0QX, United Kingdom

  • *avishek.maity@frm2.tum.de
  • †rajesh.dutta@frm2.tum.de
  • ‡werner.paulus@umontpellier.fr

Phys. Rev. B 103, L100401 – Published 2 March, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L100401

Abstract

We report an inelastic neutron scattering study on the magnetic excitations of Pr2NiO4+δ (δ∼0.24±0.01) at T=10 K. Spin stripe ordering becomes pronounced below ∼220 K with an incommensurability ε≈0.346, and a strong influence of interstitial oxygen is identified on establishing a long-range spin stripe ordering. Apart from the Goldstone modes emerging from the magnetic satellites (qm), multiple homologous modes are observed along the spin stripe modulation separated by Δqm≈0.076 in reciprocal lattice units, which is interpreted by the internal periodicity of the long-range ordered discommensurated spin stripes.

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