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Ambipolar magneto-optical response of ultralow carrier density topological insulators

Dipanjan Chaudhuri1, Maryam Salehi2,3, Sayak Dasgupta1, Mintu Mondal1,4, Jisoo Moon2, Deepti Jain2, Seongshik Oh2, and N. P. Armitage1,*

  • 1Department of Physics and Astronomy, The Johns Hopkins University, Baltimore, Maryland 21218, USA
  • 2Department of Physics and Astronomy, Rutgers, The State University of New Jersey, Piscataway, New Jersey 08854, USA
  • 3Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02138, USA
  • 4School of Physical Sciences, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032, India

  • *npa@jhu.edu

Phys. Rev. B 103, L081110 – Published 19 February, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L081110

Abstract

We have investigated the THz range magneto-optical response of ultralow carrier density films of Sb2Te3 using time-domain THz polarimetry. Undoped Sb2Te3 has a chemical potential that lies inside the bulk valence band. Thus, its topological response is masked by bulk carriers. However, with appropriate buffer-layer engineering and chemical doping, Sb2Te3 thin films can be grown with extremely low electron or hole densities. The ultralow carrier density samples show unusual optical properties and quantized response in the presence of magnetic fields. Consistent with the expectations for Dirac fermions, a quantized Hall response is seen even in samples where the zero field conductivity falls below detectable levels. The discontinuity in the Faraday angle with small changes in the filling fraction across zero is a manifestation of the parity anomaly in 2D Dirac systems with broken time reversal symmetry (TRS).

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