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Spin-orbit coupling driven orbital-selective doping effect in Sr2Ru1−xIrxO4

Junyoung Kwon1,2, Beom Seo Kim1,2, Mi Kyung Kim1,2, Jonathan Denlinger3, Aaron Bostwick3, Eli Rotenberg3, Nara Lee4, Hwan Young Choi4, Jae Young Moon4 et al.

Young Jai Choi4, Junsik Mun1,5, Miyoung Kim1,5, Yoshiyuki Yoshida6, Wonshik Kyung1,2,*, and Changyoung Kim1,2,†

  • 1Center for Correlated Electron Systems, Institute for Basic Science, Seoul 08826, Korea
  • 2Department of Physics and Astronomy, Seoul National University, Seoul 08826, Korea
  • 3Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 4Department of Physics, Yonsei University, Seoul 03722, Korea
  • 5Department of Materials Science and Engineering and Research Institute of Advanced Materials, Seoul National University, Seoul 08826, Korea
  • 6National Institute of Advanced Industrial Science and Technology, Tsukuba 305-8568, Japan

  • *specialtoss@gmail.com
  • †changyoung@snu.ac.kr

Phys. Rev. B 103, L081104 – Published 12 February, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L081104

Abstract

Orbital-selective phenomena in mutliorbital systems have received much attention due to their uniqueness as well as possible connections to other phenomena. As orbital-selectiveness is mostly related to the crystal structure, finding a new control parameter other than structure would be of significant importance. Here we report discovery of an orbital-selective doping effect in Sr2Ru1−xIrxO4 (SRIO). Our systematic electronic structure study of SRIO reveals an anomalous orbital-selective doping effect and concomitant Lifshitz transitions (LTs) in the γ band. With the help of a tight-binding calculation, we find that the orbital-selective doping effect is due to variation in the spin-orbit coupling (SOC) strength. Our findings not only elucidate the mechanism of LTs in the γ band in SRIO but may also open new avenues for novel SOC-controlled orbital-selective phenomena.

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