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Kinetic pathway facilitated by a phase competition to achieve a metastable electronic phase

Keisuke Matsuura1,*, Hiroshi Oike1,2, Vilmos Kocsis1, Takuro Sato1, Yasuhide Tomioka3, Yoshio Kaneko1, Masao Nakamura1, Yasujiro Taguchi1, Masashi Kawasaki1,2 et al.

Yoshinori Tokura1,2,4 and Fumitaka Kagawa1,2,†

  • 1RIKEN Center for Emergent Matter Science, Wako 351-0198, Japan
  • 2Department of Applied Physics and Quantum-Phase Electronics Center (QPEC), University of Tokyo, Tokyo 113-8656, Japan
  • 3National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba 305-8560, Japan
  • 4Tokyo College, University of Tokyo, Tokyo 113-8656, Japan

  • *keisuke.matsuura@riken.jp
  • †kagawa@ap.t.u-tokyo.ac.jp

Phys. Rev. B 103, L041106 – Published 14 January, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L041106

Abstract

We show that ground state phase competition significantly decreases the critical cooling rate required for the kinetic avoidance of a first-order phase transition and thus facilitates the creation of metastable electronic states. This principle is revealed for the phase transition between antiferromagnetic charge-orbital-ordered insulating and ferromagnetic metallic states in the so-called colossal magnetoresistive manganite Nd0.5Sr0.5MnO3. In a phase competition situation, we achieve reversible and nonvolatile control of bulk magnetization by 1μB/f.u. and resistivity by ∼1000% by applying electric pulses to exploit electric heating and subsequent rapid cooling.

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