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Nanosecond dynamics in intrinsic topological insulator Bi2−xSbxSe3 revealed by time-resolved optical reflectivity

Adam L. Gross1, Yasen Hou1,*, Antonio Rossi1,2, Dong Yu1,†, and Inna M. Vishik1,‡

  • 1Department of Physics and Astronomy, University of California, Davis, California 95616, USA
  • 2Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA

  • *Present address: Plasma Science and Fusion Center, Massachusetts Institute of Technology, Cambridge, MA 02139, USA.
  • †yu@physics.ucdavis.edu
  • ‡ivishik@ucdavis.edu

Phys. Rev. B 103, L020301 – Published 13 January, 2021

DOI: https://doi.org/10.1103/PhysRevB.103.L020301

Abstract

Bi2Se3 is an ideal three-dimensional topological insulator in which the chemical potential can be brought into the bulk band gap with antimony doping. Here, we utilize ultrafast time-resolved transient reflectivity to characterize the photoexcited carrier decay in Bi2−xSbxSe3 nanoplatelets. We report a substantial slowing of the bulk carrier relaxation time in bulk-insulating Bi2−xSbxSe3 as compared to n-type bulk-metallic Bi2Se3 at low temperatures, which approaches 3.3ns in the zero pump fluence limit. This long-lived decay is correlated across different fluences and antimony concentrations, revealing unique decay dynamics not present in n-type Bi2Se3, namely the slow bimolecular recombination of bulk carriers.

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