- Letter
Nanosecond dynamics in intrinsic topological insulator revealed by time-resolved optical reflectivity
Phys. Rev. B 103, L020301 – Published 13 January, 2021
DOI: https://doi.org/10.1103/PhysRevB.103.L020301
Abstract
is an ideal three-dimensional topological insulator in which the chemical potential can be brought into the bulk band gap with antimony doping. Here, we utilize ultrafast time-resolved transient reflectivity to characterize the photoexcited carrier decay in nanoplatelets. We report a substantial slowing of the bulk carrier relaxation time in bulk-insulating as compared to -type bulk-metallic at low temperatures, which approaches in the zero pump fluence limit. This long-lived decay is correlated across different fluences and antimony concentrations, revealing unique decay dynamics not present in -type , namely the slow bimolecular recombination of bulk carriers.