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Long-lived coherence between incoherent excitons revealed by time-resolved angle-resolved photoemission spectroscopy: An exact solution

Zhenlin Zhang1, Wei Hu1, Enrico Perfetto2,3, and Gianluca Stefanucci2,3

  • 1Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
  • 2Dipartimento di Fisica, Università di Roma Tor Vergata, Via della Ricerca Scientifica 1, 00133 Rome, Italy
  • 3INFN, Sezione di Roma Tor Vergata, Via della Ricerca Scientifica 1, 00133 Rome, Italy

Phys. Rev. B 111, 235124 – Published 12 June, 2025Erratum Phys. Rev. B 113, 239904 (2026)

DOI: https://doi.org/10.1103/9spx-3hrq

Abstract

We investigate the exciton dynamics in an exactly solvable two-band model for semiconductors. The model incorporates light-matter, electron-electron, and electron-phonon interactions, and captures exciton formation as well as the transition from the coherent to the incoherent regime. We analyze excitonic polarization, populations, and coherences, with special focus on their impact in time-resolved angle-resolved photoemission spectroscopy (TR-ARPES). For nonresonant pumping with below-gap photon energies, TR-ARPES spectra reveal distinct excitonic replica and quantum beats persisting in the incoherent regime. These are due to a coherence between different species of incoherent excitons. Such type of coherence is resistant to phonon dephasing, indicating that it follows different dynamics than those governing the coherences considered so far.

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