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Bulk and nanoflake transport properties in the van der Waals heavy-fermion metal CeSiI

Xinyu Chen1, Jiaxiang Ma1, Mengzhu Shi1, Wenxiang Wang2, Kaixin Tang1, Kaibao Fan1, Jiaqiang Cai2,3, Jinglei Zhang3, and Xianhui Chen1,2,4,*

  • *Contact author: chenxh@ustc.edu.cn

Phys. Rev. B 113, L161112 – Published 15 April, 2026

DOI: https://doi.org/10.1103/9ny7-qxyn

Abstract

Heavy-fermion systems have attracted extensive attention as platforms for investigating exotic quantum phenomena, ranging from quantum criticality to unconventional superconductivity. Substantial efforts have focused on modulating quantum phases by dimensional reduction, representing a long-standing challenge for conventional heavy-fermion compounds with three-dimensional crystal and electronic structures. Here, we report the transport properties of bulk and nanoflake samples of CeSiI, a van der Waals antiferromagnet that has been established as a heavy-fermion metal. Magnetic torque and magnetoresistance measurements reveal two metamagnetic transitions at μ0H≈2.4 and 4.2T. Zero-field out of plane and in-plane electronic transport measurements indicate a heavy-fermion behavior with T2-linear dependence on resistivity in the antiferromagnetic state. As the magnetic field increases, the antiferromagnetic state is gradually suppressed, and the resistivity deviates from the T2-linear relationship simultaneously; this suggests a deeper underlying coupling between the heavy-fermion behavior and the antiferromagnetic order. These two features persist down to the nanoflakes, but the metamagnetic transitions are suppressed by proton gating. Our work establishes CeSiI as an ideal platform for investigating the interplay between Kondo screening and magnetic order in bulk crystals and as a potential building block for engineering two-dimensional heterostructures.

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