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    Probing and modeling of photoexcited carrier dynamics in Ge-based heterostructures

    Brenden A. Magill1,*, Rathsara R. H. H. Mudiyanselage1,*, Thalya Paleologu2,*, Christopher E. McKinney2, Yannick Pleimling1, Nicholas W. G. Smith1, Mantu Hudait3, Christopher J. Stanton2,†, and Giti A. Khodaparast1,‡

    • 1Department of Physics, Virginia Tech, Blacksburg, Virginia 24061, USA
    • 2Department of Physics, University of Florida, Gainesville, Florida 32611, USA
    • 3Department of Electrical and Computer Engineering, Virginia Tech, Blacksburg, Virginia 24061, USA

    • *These authors contributed equally to this work.
    • †Contact author: stanton@phys.ufl.edu
    • ‡Contact author: khoda@vt.edu

    Phys. Rev. B 112, 075308 – Published 29 August, 2025

    DOI: https://doi.org/10.1103/92r8-d4dr

    Abstract

    While germanium (Ge) has long been an important player in microelectronics, strain-engineered Ge heterostructures have recently gained increased attention owing to the intriguing possibility of using strain to change the relative positions of the conduction band valleys and, as a result, go from an indirect to a direct gap material. Time-resolved pump-probe spectroscopy is an excellent tool to provide insight into the fundamental interactions and microscopic dynamics of electrons, holes, phonons, and impurities. In this study, using complementary techniques of single-color time-resolved differential reflectivity and two-color time-resolved differential transmission, we gained insights into the effects of interfacial strain on carrier dynamics in several different Ge-based heterostructures. Our structures include high-quality Ge films interfaced with InGaAs and AlAs grown on semi-insulating GaAs as the substrate. In contrast to traditional microwave photoconductivity decay (μ−PCD) measurements, which typically have a time resolution on the ns scale, we probe samples on a 100 fs scale and can measure decay times approximately three orders of magnitude faster than previous μ−PCD measurements. Therefore, our results are sensitive to the effects of both carrier recombination as well as electron intervalley and hole interband scattering.

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