Probing and modeling of photoexcited carrier dynamics in Ge-based heterostructures
Phys. Rev. B 112, 075308 – Published 29 August, 2025
DOI: https://doi.org/10.1103/92r8-d4dr
Abstract
While germanium (Ge) has long been an important player in microelectronics, strain-engineered Ge heterostructures have recently gained increased attention owing to the intriguing possibility of using strain to change the relative positions of the conduction band valleys and, as a result, go from an indirect to a direct gap material. Time-resolved pump-probe spectroscopy is an excellent tool to provide insight into the fundamental interactions and microscopic dynamics of electrons, holes, phonons, and impurities. In this study, using complementary techniques of single-color time-resolved differential reflectivity and two-color time-resolved differential transmission, we gained insights into the effects of interfacial strain on carrier dynamics in several different Ge-based heterostructures. Our structures include high-quality Ge films interfaced with InGaAs and AlAs grown on semi-insulating GaAs as the substrate. In contrast to traditional microwave photoconductivity decay () measurements, which typically have a time resolution on the ns scale, we probe samples on a 100 fs scale and can measure decay times approximately three orders of magnitude faster than previous measurements. Therefore, our results are sensitive to the effects of both carrier recombination as well as electron intervalley and hole interband scattering.