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    Strain-induced nonrelativistic altermagnetic spin splitting effect

    Wancheng Zhang1,2, Mingkun Zheng1,2, Yong Liu3, Zhenhua Zhang1,2,*, Rui Xiong3,†, and Zhihong Lu1,2,‡

    • *Contact author: zzhua@wust.edu.cn
    • †Contact author: xiongrui@whu.edu.cn
    • ‡Contact author: zludavid@live.com

    Phys. Rev. B 112, 024415 – Published 10 July, 2025

    DOI: https://doi.org/10.1103/8zlt-mlms

    Abstract

    Recent studies reveal that T-odd spin currents generated via the nonrelativistic altermagnetic spin splitting effect (ASSE) exhibit significant potential for spintronics applications, with both computational and experimental validations. Addressing the scarcity of conductive altermagnets, we propose strain engineering as a reliable method for inducing altermagnetism. Focusing on rutile-structured OsO2, first-principles calculations show that minor equibiaxial tensile strain (Ets=3%) induces nonmagnetic-to-altermagnetic transitions, achieving an ASSE-driven spin-charge conversion ratio (θAS) of ∼7%—far surpassing conventional spin Hall angles (θIS). Calculations reveal that substantial θAS persists even in the absence of spin-orbit coupling, with its magnitude positively correlating to nonrelativistic spin splitting magnitude, which further confirms the strain-induced ASSE's nonrelativistic origin. Further investigation reveals that RuO2 exhibits analogous phenomena, which may resolve recent controversies regarding its magnetic properties. Our research opens new simple pathways for developing next-generation altermagnetic spintronics devices.

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