High spin, low spin, or gapped spins: Magnetism in the bilayer nickelates
Phys. Rev. B 113, 024430 – Published 26 January, 2026
DOI: https://doi.org/10.1103/8s6y-vcch
Abstract
Inspired by the recent discovery of high-temperature superconductivity in bilayer nickelates, we investigate the role of magnetism emerging from a hypothetical insulating parent state. We demonstrate that due to the interplay of superexchange and Hund's coupling, the system can be in a high-spin, low-spin, or spin-gapped state. The low-spin state has singlets across the bilayer in the orbital, with charge carriers in the orbital. Thus, at low energy scales, it behaves as an effective one-band system when hole doped. By contrast, the high-spin state is a more robust, spin-1 antiferromagnet. Using Hartree-Fock methods, we find that for fixed interaction strength and doping, high-spin magnetism remains more robust than the low-spin counterpart. Whether this implies that the high-spin state provides a stronger pairing glue or more strongly competes with superconductivity remains an open question. Our analysis, therefore, underscores the importance of identifying the spin state for understanding superconductivity in nickelates.