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    High spin, low spin, or gapped spins: Magnetism in the bilayer nickelates

    Hanbit Oh1,*, Yi-Ming Wu2,*, Julian May-Mann3, Yijun Yu4,5, Harold Y. Hwang4,5, Ya-Hui Zhang1,†, and S. Raghu2,4,‡

    • *These authors contributed equally to this work.
    • †Contact author: yzhan566@jhu.edu
    • ‡Contact author: sraghu@stanford.edu

    Phys. Rev. B 113, 024430 – Published 26 January, 2026

    DOI: https://doi.org/10.1103/8s6y-vcch

    Abstract

    Inspired by the recent discovery of high-temperature superconductivity in bilayer nickelates, we investigate the role of magnetism emerging from a hypothetical insulating d8 parent state. We demonstrate that due to the interplay of superexchange and Hund's coupling, the system can be in a high-spin, low-spin, or spin-gapped state. The low-spin state has singlets across the bilayer in the dz2 orbital, with charge carriers in the dx2−y2 orbital. Thus, at low energy scales, it behaves as an effective one-band system when hole doped. By contrast, the high-spin state is a more robust, spin-1 antiferromagnet. Using Hartree-Fock methods, we find that for fixed interaction strength and doping, high-spin magnetism remains more robust than the low-spin counterpart. Whether this implies that the high-spin state provides a stronger pairing glue or more strongly competes with superconductivity remains an open question. Our analysis, therefore, underscores the importance of identifying the spin state for understanding superconductivity in nickelates.

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