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    Magnetization flip caused by magnetic field rotation in compensated Ni4Nb2O9 ferrimagnet with exchange bias

    I. Fita1,*, R. Puzniak1, E. E. Zubov2, C. Martin3, A. Maignan3, and A. Wisniewski1

    • *Contact author: ifita@ifpan.edu.pl

    Phys. Rev. B 114, 194429 – Published 29 October, 2026

    DOI: https://doi.org/10.1103/8pjy-d3tz

    Abstract

    A single-crystal compensated ferrimagnet Ni4Nb2O9, consisting of two antiferromagnetically coupled ferromagnetic (FM) Ni2+ layers with opposite moments in the ab plane, exhibiting noninterface exchange bias (EB), was investigated. The magnetization hysteresis loops M(θ), measured at a weak field H rotating in FM layers clockwise and then counterclockwise, show two successive M flips in opposite directions with a large hysteresis of the flip angle θMR. It was found that the angle θMR shifts due to EB to higher or lower values, depending on the sign of the unidirectional anisotropy EB specified by the field cooling protocol. Furthermore, the EB effect also influences the temperature of spontaneous switching Tsw from negative to positive magnetization, which occurs below Tcomp=33K, at a constant field H. Namely, Tsw decreases in the presence of positive unidirectional anisotropy and increases in the presence of negative anisotropy, indicating that the energy required to flip M depends on the sign of EB. The features discovered allow us to more fully comprehend the nature of the EB effect in coupled FM layers of compensated Ni4Nb2O9 ferrimagnet.

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