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  • Letter

Nonreciprocal magnons in layered antiferromagnets VPX3 (X=S,Se,Te)

Quanchao Du1,*, Zhenlong Zhang1,*, Jinyang Ni1,2,†, Zhijun Jiang1,2,‡, and Laurent Bellaiche3,4

  • 1Ministry of Education Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter, Shaanxi Province Key Laboratory of Advanced Functional Materials and Mesoscopic Physics, School of Physics, Xi'an Jiaotong University, Xi'an 710049, China
  • 2Key Laboratory of Computational Physical Sciences (Ministry of Education), Institute of Computational Physical Sciences, State Key Laboratory of Surface Physics and Department of Physics, Fudan University, Shanghai 200433, China
  • 3Smart Ferroic Materials Center, Department of Physics and Institute for Nanoscience and Engineering, University of Arkansas, Fayetteville, Arkansas 72701, USA
  • 4Department of Materials Science and Engineering, Tel Aviv University, Ramat Aviv, Tel Aviv 6997801, Israel

  • *These authors contributed equally to this work.
  • †Contact author: jyni18@fudan.edu.cn
  • ‡Contact author: zjjiang@xjtu.edu.cn

Phys. Rev. B 112, L100408 – Published 19 September, 2025

DOI: https://doi.org/10.1103/8fx7-4xgm

Abstract

Nonreciprocal magnons, characterized by propagation with differing energies along the k and −k directions, are crucial for modern spintronics applications. However, their realization in van der Waals layered antiferromagnets remains elusive. In this Letter, we report robust nonreciprocal magnon behavior in layered honeycomb antiferromagnets VPX3 (X=S, Se, Te). Our results demonstrate that, in addition to their intrinsic Dzyaloshinsky-Moriya interaction, the nonreciprocity of magnons is strongly influenced by the layer number, interlayer coupling, and magnon-magnon interactions. More importantly, in such layered antiferromagnets, the magnon nonreciprocity exhibits an asymmetric periodic dependence on the Néel vector, offering a novel route for experimentally probing antiferromagnetic order parameters in the two-dimensional limit.

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