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    Dual-switch control of a layer-locked anomalous valley Hall effect in a sliding ferroelectric antiferromagnet

    Quan Shen1, Wenhu Liao1, Degao Xu2, Jiansheng Dong1,*, and Jianing Tan1,†

    • *Contact author: jsdong@jsu.edu.cn
    • †Contact author: jianing_tan@163.com

    Phys. Rev. B 113, 184407 – Published 4 May, 2026

    DOI: https://doi.org/10.1103/88tx-k9f4

    Abstract

    The integration of ferroelectric (FE) and antiferromagnetic (AFM) orders in two-dimensional (2D) materials provides a promising avenue for the nonvolatile control of coupled spin and valley degrees of freedom, a capability central to advancing spin-valleytronics. However, realizing a single material system where these quantum states can be independently and reversibly manipulated by distinct stimuli, a prerequisite for multifunctional devices, has remained elusive. Here, we demonstrate a dual-switch mechanism in bilayer VS2, a room-temperature FE-AFM system, that enables electrical and magnetic control of a layer-locked anomalous valley Hall effect (AVHE). First-principles calculations reveal that interlayer sliding breaks spatial inversion symmetry, inducing a switchable out-of-plane FE polarization that coexists with interlayer AFM. The spin-orbit coupled valley polarization can be reversibly switched either by FE polarization reversal or by a magnetic-field-induced spin-flip transition, confirming the existence of electrically and magnetically addressable valley states. The Berry curvature exhibits both valley-contrasting and layer-locked characteristics, which underpin a switchable Hall response. Notably, electric and magnetic switching are functionally equivalent in modulating valley, layer, and spin indices, revealing strong magnetoelectric coupling. This work establishes a multidegree-of-freedom operational paradigm in 2D multiferroics and opens a viable design pathway toward multistate memory and spin-valleytronic logic devices.

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