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    de Haas–van Alphen effect in the Ti-doped CsV3Sb5 kagome compound under magnetic fields up to 41 Tesla

    Kyryl Shtefiienko1, Tucker Beekmann1, Matthew J. Stitz2, Ganesh Pokharel2, Stephen D. Wilson3, Christopher A. Mizzi4, David E. Graf5,6, and Keshav Shrestha1,*

    • *Contact author: kshrestha@wtamu.edu

    Phys. Rev. B 113, 035119 – Published 9 January, 2026

    DOI: https://doi.org/10.1103/871s-2rsl

    Abstract

    The recently discovered kagome superconductor CsV3Sb5 exhibits a rich interplay between superconductivity (SC) and charge density wave order, both of which are highly tunable via doping or pressure. In particular, hole doping CsV3Sb5 by substituting vanadium with the relatively smaller titanium allows controlled tuning of the correlated phases, revealing two distinct superconducting domes (SC I and SC II) across the doping range. A prior tunneling experiment [H. Yang, et al., Sci. Bull. 67, 2176 (2022)] suggests differing SC pairing symmetries between the two domes. Since the Fermi surface topology—including features such as pockets, nesting vectors, and dimensionality—plays a crucial role in determining the superconducting pairing mechanism, we investigate its evolution in CsTixV3−xSb5 across four doping levels (x=0, 0.03, 0.10, and 0.15), spanning both SC domes. High-field torque magnetometry up to 41 T reveals pronounced de Haas–van Alphen (dHvA) oscillations, with distinct frequency spectra observed in SC I and SC II, implying that these SC domes have different electronic and Fermi surface properties. First-principles calculations using density functional theory also show changes in key electronic features—such as Dirac crossings, van Hove singularities, and flat bands—when vanadium is replaced with titanium. Notably, the Fermi surface topology shows clear deformation with increasing titanium doping. Our experimental and theoretical results provide compelling evidence for distinct Fermi surface characteristics in the SC I and SC II regions, offering insights into the possible existence of different pairing mechanisms across the two superconducting domes in CsTixV3−xSb5.

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