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    Chiral geometry driven chiral magnetism

    Yonglong Ga1,*, Dongxing Yu2,*, Jiawei Jiang1, Liming Wang1, Fengjun Zhuo1, Kai Chang1,†, and Hongxin Yang1,‡

    • 1Center for Quantum Matter, School of Physics, Zhejiang University, Hangzhou 310058, China
    • 2Key Laboratory of Magnetism and Magnetic Functional Materials of MoE, Lanzhou University, Lanzhou 730000, China

    • *These authors contributed equally to this work.
    • †Contact author: kchang@zju.edu.cn
    • ‡Contact author: hongxin.yang@zju.edu.cn

    Phys. Rev. B 113, 024403 – Published 5 January, 2026

    DOI: https://doi.org/10.1103/81rn-9t23

    Abstract

    We extend the study of topological magnetisms to quasi-one-dimensional chiral geometries, revealing a symmetry-guided pathway to Dzyaloshinskii–Moriya interactions (DMI) and enabling the design of high-density spintronic devices. Utilizing symmetry analysis, a general strategy is proposed for inducing Bloch-type DMI in chiral geometries warped by low-dimensional magnets. By combining first-principles calculations, we demonstrate our concept in various chiral geometries, e.g., chiral nanoribbon and nanotubes, which are composed of quasi-one-dimensional CrBr2 nanoribbon and two-dimensional magnets with different crystal symmetries, including CrN, transition metal dichalcogenides, VSe, CrI3, and Cr2Se3. More interestingly, we find that the chirality of Bloch-type DMI can be closely coupled with the helical direction of the chiral geometry. Our atomistic spin dynamics study using Monte Carlo simulation is performed on chiral VS2 nanotube as an example, in which Bloch-type domain walls with opposite chirality arising from Bloch-type DMI can be stabilized via opposite chirality indices (n, m) and (m, n). Our results that chiral geometry induces DMI in a broad range of 2D magnets, enabling topological magnetisms, pave the way for the development of geometry-driven spintronic devices.

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