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    Theoretical investigation of electronic structure and magnetism in the kagome material CsCr3Sb5

    Wei Wang1,2, Shun-Li Yu3,4,*, and Jian-Xin Li3,4,†

    • *Contact author: slyu@nju.edu.cn
    • †Contact author: jxli@nju.edu.cn

    Phys. Rev. B 112, 165137 – Published 23 October, 2025

    DOI: https://doi.org/10.1103/7mc7-x9ky

    Abstract

    Kagome quantum materials, with their frustrated lattice geometry and flat-band electronic structure, serve as a versatile platform for studying magnetism and electron correlation. The recently discovered kagome metal CsCr3Sb5 has garnered significant interest for its coexistence of multiple orders and the emergence of pressure-induced superconductivity. In this study, we theoretically investigate the correlation effects on the electronic structures and magnetism of CsCr3Sb5. Based on our proposed effective tight-binding model, we reveal orbital-selective correlation effects that induce a near-flat band just below the Fermi level, consistent with recent experimental observations. By combining the symmetry analysis and second-order perturbation theory, we construct an effective spin model and thoroughly explore its classical phase diagram, suggesting that a special q=0 state might correspond to the magnetic order in CsCr3Sb5. Our findings highlight the electron correlations in CsCr3Sb5 and provide novel insights into its magnetic properties. Furthermore, this spin model is applicable to kagome materials with similar structures, making the complete phase diagram relevant to other similar systems as well.

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