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    Higher-order topological insulators in two-dimensional antiferromagnetic and altermagnetic chromium-based group-IV chalcogenides

    Ruo-Yu Ning1, Yong-Kun Wang1, Shifeng Qian2, Si Li1,3,4,5,*, and Wen-Li Yang3,4,5,6

    • 1School of Physics, Northwest University, Xi'an 710127, China
    • 2Anhui Province Key Laboratory for Control and Applications of Optoelectronic Information Materials, Department of Physics, Anhui Normal University, Wuhu, Anhui 241000, China
    • 3Shaanxi Key Laboratory for Theoretical Physics Frontiers, Xi'an 710127, China
    • 4Peng Huanwu Center for Fundamental Theory, Xi'an 710127, China
    • 5Fundamental Discipline Research Center for Quantum Science and Technology of Shaanxi Province, Xi'an 710127, China
    • 6Institute of Modern Physics, Northwest University, Xi'an 710127, China

    • *Contact author: sili@nwu.edu.cn

    Phys. Rev. B 113, 165114 – Published 9 April, 2026

    DOI: https://doi.org/10.1103/7dnk-crq7

    Abstract

    Based on first-principles calculations combined with theoretical analysis, we identify a family of monolayer chromium-based group-IV chalcogenides as a new class of two-dimensional (2D) magnetic higher-order topological insulators (HOTIs). Specifically, the CrCX3 (X=S, Se, Te) and CrSiS3 monolayers are found to host conventional antiferromagnetic ground states with PT symmetry, whereas the Janus compounds Cr2C2S3Se3 and Cr2Si2S3Se3 exhibit altermagnetic ground states. We demonstrate that all these monolayer magnetic materials realize 2D HOTI phases, in which the nontrivial topology is protected by lattice C3 rotational symmetry and manifests as zero-dimensional corner states carrying quantized fractional charges. Moreover, upon inclusion of spin-orbit coupling, these systems remain in the HOTI phase and continue to host robust corner-localized states, confirming the stability of their higher-order topological nature. Our results reveal an intrinsic connection between higher-order topology and magnetic order in 2D antiferromagnetic and altermagnetic systems, identifying chromium-based group-IV chalcogenide monolayers as promising platforms for exploring higher-order topological phases and their potential relevance for future topological and spintronic applications.

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