Extremely large magnetoresistance and Shubnikov-de Haas oscillations in topological semimetal
Phys. Rev. B 112, 115149 – Published 26 September, 2025
DOI: https://doi.org/10.1103/6ycd-k56z
Abstract
Extremely large magnetoresistance (XMR) observed in topological materials holds significant promise for spintronic applications. In this work, we systematically investigate the magnetotransport properties and quantum oscillations in high-quality single crystals of the magnetic nodal-line semimetal . Synthesized via chemical vapor transport, the crystals exhibit an exceptional residual resistivity ratio of 533 and achieve a nonsaturating XMR of at 1.8 K and 14 T, accompanied by ultrahigh carrier mobility (). Shubnikov-de Haas oscillations reveal a -Berry phase, suggesting a possible nontrivial topological nature of . The remarkably high ratio of transport-to-quantum lifetimes () further confirms suppression of backscattering, possibly related to topological protection. Combined with Hall effect measurements and extended Kohler scaling analysis, we establish that the origin of XMR in arises from the synergistic interplay between topological protection and high carrier mobility, rather than conventional electron-hole compensation. These findings not only provide critical experimental insights into the XMR mechanism of magnetic nodal-line semimetals but also highlight as a promising candidate for designing next-generation topological spintronic devices.