Persistent short-range spin fluctuation in rare-earth substituted square lattice
Phys. Rev. B 112, 144430 – Published 16 October, 2025
DOI: https://doi.org/10.1103/6nxd-77m2
Abstract
, a prototypical square lattice system, is widely studied for novel physics. While transition metal substitution effects are well explored, rare-earth doping at the site is less explored. Here we present a detailed magnetization and neutron diffraction study on . The system tends to adopt an in-plane antiferromagnetic configuration with a “” stacking sequence. Strong spin fluctuations persist down to the lowest measured temperature, consistent with the concave shape order parameter. A pronounced magnetic diffuse scattering rod develops along the direction at low temperature, indicating the formation of short-range magnetic correlations with a characteristic length of . This work provides a new pathway to exotic quantum phases in the strongly spin-orbit-coupled iridates.