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    Persistent short-range spin fluctuation in rare-earth substituted square lattice Sr2Ir0.89Tb0.11O4

    Jiasen Guo1, Jieming Sheng1,*, Zachary Morgan1, Masaaki Matsuda1, Gang Cao2, and Feng Ye1,†

    • *Present address: School of Physical Sciences, Great Bay University and Great Bay Institute for Advanced Study, Dongguan 523000, China.
    • †Contact author: 2fy@ornl.gov

    Phys. Rev. B 112, 144430 – Published 16 October, 2025

    DOI: https://doi.org/10.1103/6nxd-77m2

    Abstract

    Sr2IrO4, a prototypical Jeff=1/2 square lattice system, is widely studied for novel physics. While transition metal substitution effects are well explored, rare-earth doping at the Ir4+ site is less explored. Here we present a detailed magnetization and neutron diffraction study on Sr2Ir1−xTbxO4 (x=0.11). The system tends to adopt an in-plane antiferromagnetic configuration with a “++++” stacking sequence. Strong spin fluctuations persist down to the lowest measured temperature, consistent with the concave shape order parameter. A pronounced magnetic diffuse scattering rod develops along the L direction at low temperature, indicating the formation of short-range magnetic correlations with a characteristic length of ∼24(2)Å. This work provides a new pathway to exotic quantum phases in the strongly spin-orbit-coupled iridates.

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